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1.
Nano Lett ; 23(24): 11727-11733, 2023 Dec 27.
Artigo em Inglês | MEDLINE | ID: mdl-38014963

RESUMO

We demonstrated optical bistability in an amorphous silicon Mie resonator with a size of ∼100 nm and Q-factor as low as ∼4 by utilizing photothermal and thermo-optical effects. We not only experimentally confirmed the steep intensity transition and the hysteresis in the scattering response from silicon nanocuboids but also established a physical model to numerically explain the underlying mechanism based on temperature-dependent competition between photothermal heating and heat dissipation. The transition between the bistable states offered particularly steep superlinearity of scattering intensity, reaching an effective nonlinearity order of ∼100th power over excitation intensity, leading to the potential of advanced optical switching devices and super-resolution microscopy.

2.
Adv Sci (Weinh) ; 10(30): e2302707, 2023 Oct.
Artigo em Inglês | MEDLINE | ID: mdl-37661570

RESUMO

2D materials have manifested themselves as key components toward compact integrated circuits. Because of their capability to circumvent the diffraction limit, light manipulation using surface plasmon polaritons (SPPs) is highly-valued. In this study, plasmonic photodetection using graphene as a 2D material is investigated. Non-scattering near-field detection of SPPs is implemented via monolayer graphene stacked under an SPP waveguide with a symmetric antenna. Energy conversion between radiation power and electrical signals is utilized for the photovoltaic and photoconductive processes of the gold-graphene interface and biased electrodes, measuring a maximum photoresponsivity of 29.2 mA W-1 . The generated photocurrent is altered under the polarization state of the input light, producing a 400% contrast between the maximum and minimum signals. This result is universally applicable to all on-chip optoelectronic circuits.

3.
ACS Appl Mater Interfaces ; 14(26): 30299-30305, 2022 Jul 06.
Artigo em Inglês | MEDLINE | ID: mdl-35675390

RESUMO

Recently, nanoscale light manipulation using surface plasmon polaritons (SPPs) has received considerable research attention. The conventional method of detecting SPPs is through light scattering or using bulky Si or Ge photodetectors. However, these bulky systems limit the application of nanophotonic circuits. In this study, the light-matter interaction between graphene and SPP was investigated. For realizing an improved integration in nanocircuits, single-layer graphene was added to asymmetric SPP nanoantenna arrays for nonscattering detection in the near field. The developed device is capable of detecting the controlled propagation of SPPs with a photoresponsivity of 15 mA/W, which paves the way for the new-generation on-chip optical communication.

4.
ACS Nano ; 16(4): 5994-6001, 2022 Apr 26.
Artigo em Inglês | MEDLINE | ID: mdl-35191683

RESUMO

In O-and C-band optical communications, Ge is a promising material for detecting optical signals that are encoded into electrical signals. Herein, we study 2D periodic Ge metasurfaces that support optically induced electric dipole and magnetic dipole lattice resonances. By overlapping Mie resonances and electric dipole lattice resonances, we realize the resonant lattice Kerker effect and achieve narrowband absorption. This effect was applied to the photodetector demonstrated in this study. The absorptance of the Ge nanoantenna arrays increased 6-fold compared to that of the unpatterned Ge films. In addition, the photocurrent in such Ge metasurface photodetectors increases by approximately 5 times compared with that in plane Ge film photodetectors by the interaction of these strong near-fields with semiconductors and the further transformation of the optical energy into electricity.

5.
Materials (Basel) ; 14(11)2021 May 24.
Artigo em Inglês | MEDLINE | ID: mdl-34073879

RESUMO

Chiral-selective Tamm plasmon polariton (TPP) has been investigated at the interface between a cholesteric liquid crystal and a metasurface. Different from conventional TPP that occurs with distributed Bragg reflectors and metals, the chiral-achiral TPP is successfully demonstrated. The design of the metasurface as a reflective half-wave plate provides phase and polarization matching. Accordingly, a strong localized electric field and sharp resonance are observed and proven to be widely tunable.

7.
Nat Commun ; 11(1): 4101, 2020 Aug 14.
Artigo em Inglês | MEDLINE | ID: mdl-32796839

RESUMO

Silicon photonics have attracted significant interest because of their potential in integrated photonics components and all-dielectric meta-optics elements. One major challenge is to achieve active control via strong photon-photon interactions, i.e. optical nonlinearity, which is intrinsically weak in silicon. To boost the nonlinear response, practical applications rely on resonant structures such as microring resonators or photonic crystals. Nevertheless, their typical footprints are larger than 10 µm. Here, we show that 100 nm silicon nano-resonators exhibit a giant photothermal nonlinearity, yielding 90% reversible and repeatable modulation from linear scattering response at low excitation intensities. The equivalent nonlinear index is five-orders larger compared with bulk, based on Mie resonance enhanced absorption and high-efficiency heating in thermally isolated nanostructures. Furthermore, the nanoscale thermal relaxation time reaches nanosecond. This large and fast nonlinearity leads to potential applications for GHz all-optical control at the nanoscale and super-resolution imaging of silicon.

8.
ACS Nano ; 14(5): 5678-5685, 2020 May 26.
Artigo em Inglês | MEDLINE | ID: mdl-32298575

RESUMO

Artificial color pixels based on dielectric Mie resonators are appealing for scientific research as well as practical design. Vivid colors are imperative for displays and imaging. Dielectric metasurface-based artificial pixels are promising candidates for developing flat, flexible, and/or wearable displays. Considering the application feasibility of artificial color pixels, wide color gamuts are crucial for contemporary display technology. To achieve a wide color gamut, ensuring the purity and efficiency of nanostructure resonance peaks in the visible spectrum is necessary for structural color design. Low-loss dielectric materials are suitable for achieving vivid colors with structural color pixels. However, high-order Mie resonances prevent color pixels based on dielectric metasurfaces from efficiently generating highly saturated colors. In particular, fundamental Mie resonances (electric/magnetic dipole) for red can result in not only a strong resonance peak at 650 nm but also high-order Mie resonances at shorter wavelengths, which reduces the saturation of the target color. To address these problems, we fabricated silicon nitride metasurfaces on quartz substrates and applied Rayleigh anomalies at relatively short wavelengths to successfully suppress high-order Mie resonances, thus creating vivid color pixels. We performed numerical design, semianalytic considerations, and experimental proof-of-concept examinations to demonstrate the performance of the silicon nitride metasurfaces. Apart from traditional metasurface designs that involve transmission and reflection modes, we determined that lateral light incidence on silicon nitride metasurfaces can provide vivid colors through long-range dipole interactions; this can thus extend the applications of such surfaces to eyewear displays and guided-wave illumination techniques.

9.
Sci Rep ; 9(1): 11778, 2019 Aug 13.
Artigo em Inglês | MEDLINE | ID: mdl-31409844

RESUMO

The near-field coupling between a high-refractive-index nanoparticle and gold nanoantennas is investigated theoretically. The absorption enhancement and also avoided resonance crossing in the absorption cross section spectra were observed with the hybridization system due to the coupling between the localized surface plasmon resonance of the gold nanoantennas and the magnetic dipole resonance of the silicon nanoparticle. By controlling the nanoparticle size or the separation distance, the near-field coupling can be tuned from the weak to the strong regime.

10.
Nano Lett ; 19(8): 5017-5024, 2019 Aug 14.
Artigo em Inglês | MEDLINE | ID: mdl-31268338

RESUMO

Graphene is a two-dimensional (2D) structure that creates a linear relationship between energy and momentum that not only forms massless Dirac fermions with extremely high group velocity but also exhibits a broadband transmission from 300 to 2500 nm that can be applied to many optoelectronic applications, such as solar cells, light-emitting devices, touchscreens, ultrafast photodetectors, and lasers. Although the plasmonic resonance of graphene occurs in the terahertz band, graphene can be combined with a noble metal to provide a versatile platform for supporting surface plasmon waves. In this study, we propose a hybrid graphene-insulator-metal (GIM) structure that can modulate the surface plasmon polariton (SPP) dispersion characteristics and thus influence the performance of plasmonic nanolasers. Compared with values obtained when graphene is not used on an Al template, the propagation length of SPP waves can be increased 2-fold, and the threshold of nanolasers is reduced by 50% when graphene is incorporated on the template. The GIM structure can be further applied in the future to realize electrical control or electrical injection of plasmonic devices through graphene.

11.
Nano Lett ; 18(2): 747-753, 2018 02 14.
Artigo em Inglês | MEDLINE | ID: mdl-29320208

RESUMO

Concentrating light at the deep subwavelength scale by utilizing plasmonic effects has been reported in various optoelectronic devices with intriguing phenomena and functionality. Plasmonic waveguides with a planar structure exhibit a two-dimensional degree of freedom for the surface plasmon; the degree of freedom can be further reduced by utilizing metallic nanostructures or nanoparticles for surface plasmon resonance. Reduction leads to different lightwave confinement capabilities, which can be utilized to construct plasmonic nanolaser cavities. However, most theoretical and experimental research efforts have focused on planar surface plasmon polariton (SPP) nanolasers. In this study, we combined nanometallic structures intersecting with ZnO nanowires and realized the first laser emission based on pseudowedge SPP waveguides. Relative to current plasmonic nanolasers, the pseudowedge plasmonic lasers reported in our study exhibit extremely small mode volumes, high group indices, high spontaneous emission factors, and high Purell factors beneficial for the strong interaction between light and matter. Furthermore, we demonstrated that compact plasmonic laser arrays can be constructed, which could benefit integrated plasmonic circuits.

12.
Opt Express ; 25(24): 30764-30770, 2017 Nov 27.
Artigo em Inglês | MEDLINE | ID: mdl-29221102

RESUMO

Designing color pixels using plasmonic nanostructures and metasurfaces has become a luring area of research in recent years. Here, we experimentally demonstrated the voltage tunability of a dynamic plasmonic color filter by using an aluminum grating integrated with the nematic liquid crystal (LC). Along with a typical substrate coated with rubbed polyimide film, the aluminum grating itself serves as a molecular alignment layer to form a twisted LC cell. This hybrid structure allows electrically controlled transmission color by applying the voltage. A significant spectral tunability of such a device has been demonstrated by applying the small voltage from 0 to 4 Vrms.

13.
Sci Rep ; 6: 32194, 2016 09 01.
Artigo em Inglês | MEDLINE | ID: mdl-27581766

RESUMO

Symmetry-breaking and scattering cancellation were observed in the dark-mode resonance of dipolar gold nanoantennas (NAs) on glass substrates coupled with oblique incidence and total internal reflection. With the assistance of evanescent waves, the coupling efficiency was twice as strong when the incidence angle was larger than the critical angle. The Hamiltonian equation and absorption spectra were used to analyze the hybridization model of symmetric dipolar gold NAs. The antibonding mode could be coupled successfully by both transverse-magnetic (TM) and transverse-electric (TE) polarizations to NAs when the dimers orientation is parallel to the propagation direction of evanescent waves.

14.
PLoS One ; 8(2): e55795, 2013.
Artigo em Inglês | MEDLINE | ID: mdl-23383347

RESUMO

The expression of cytokines, such as IL-1ß, and the activation of the epidermal growth factor receptor (EGFR) are crucial regulators in the process of carcinogenesis. The correlation between growth factor and activated cytokine signals in the control of tumor development is a critical issue to be clarified. In our study, we found that the IL-1ß gene and protein expression were induced by EGF in squamous cell carcinoma. To clarify the mechanism involved in EGF-regulated IL-1ß expression, we examined the transcriptional activity and mRNA stability of IL-1ß in EGF-treated cells. We found that EGF induced the expression of IL-1ß and was mediated through transcriptional activation, but not through mRNA stability. The involvement of Akt and NF-κB signaling pathways in the EGF-induced IL-1ß gene expression was confirmed by knockdown of RelA and Akt in cells or treating cells with Akt and NF-κB inhibitors, LY294002 and parthenolide, respectively. The expression of dominant negative IκB also repressed the activation of NF-κB and inhibited EGF-induced IL-1ß expression. Using immunofluorescence staining assay, the EGF-stimulated nuclear translocation of NF-κB (p65) was inhibited by pre-treating cells with LY294002 and parthenolide. Furthermore, EGF increased the binding of NF-κB to the NF-κB binding site of the IL-1ß promoter through the activation of the Akt/NF-κB pathway, which resulted in activating IL-1ß promoter activity. The expression and secretion of IL-1ß induced by EGF considerably reduced chemotherapeutic drug cisplatin-induced cell death. These results showed that EGF enhanced the expression of IL-1ß, which was mediated by the Akt/NF-κB pathway. The activation of EGF signaling and increase of IL-1ß contributed to chemotherapeutic resistance of cancer cells, suggesting that the expression of IL-1ß may be used as a biomarker to evaluate successful cancer treatment.


Assuntos
Biomarcadores Tumorais/metabolismo , Carcinoma de Células Escamosas/metabolismo , Cisplatino/farmacologia , Citotoxinas/farmacologia , Fator de Crescimento Epidérmico/metabolismo , Regulação Neoplásica da Expressão Gênica/fisiologia , Interleucina-1beta/metabolismo , Western Blotting , Carcinoma de Células Escamosas/tratamento farmacológico , Cromonas , Cisplatino/metabolismo , Citotoxinas/metabolismo , Primers do DNA/genética , Ensaio de Imunoadsorção Enzimática , Receptores ErbB/metabolismo , Citometria de Fluxo , Imunofluorescência , Humanos , Morfolinas , NF-kappa B/metabolismo , Proteína Oncogênica v-akt/metabolismo , Interferência de RNA , RNA Interferente Pequeno/genética , Reação em Cadeia da Polimerase em Tempo Real , Reação em Cadeia da Polimerase Via Transcriptase Reversa , Sesquiterpenos , Transdução de Sinais/genética , Transdução de Sinais/fisiologia
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